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81.
Qianyu Yang Chen Gao Xuemei Zhang Xingyu Zhao Yiqing Fu Chihui Tsou Chunyan Zeng Li Yuan Zejun Pu Yiqing Xia Yuping Sheng Yu Fang 《应用聚合物科学杂志》2021,138(13):50308
Shape memory hydrogels (SMHs) can fix the hydrogels in a provisional shape and restore the initial shape under external stimulation. Herein, a dual-responsive shape memory hydrogel with dual-responsive swelling and self-healing properties is presented in this work. The SMHs were fabricated by one-step emulsion copolymerization of acrylic acid (AAc), acrylamide (AAm) and stearyl methacrylate (SMA). Sodium alginate (SA) was introduced as an interpenetrating polymer in the network. With ionic cross-linking between -COO− and Fe3+ or saline-reinforced hydrophobic association, the hydrogels can be fixed in a provisional shape, which can be restored by immersing the hydrogels in vitamin C solution or pure water, respectively. When the as-prepared hydrogels were immersed in FeCl3 solutions, additional ionic cross-linking between Fe3+ and -COO− could be formed, thus constructing the dual physically cross-linked (DPC) network, which endows the hydrogels with excellent fracture stress (2.6 MPa) and toughness (5.47 MJ/m3). Besides, the reversible physical cross-linkings endowed the hydrogel with outstanding self-healing capability. Furthermore, the pH and saline responsive swelling properties of the SMHs are additional fantastic properties. Therefore, we believe that this simple strategy provides a great opportunity for the preparation of SMHs with multiple intellectual performances. 相似文献
82.
Maolan Zhang Yuanliang Wang Guoming Zeng Shuang Yang Xiaoling Liao Da Sun 《应用聚合物科学杂志》2021,138(20):50451
Piperazine polymers poly(ethylenediaminetetraacetic dianhydride-co-piperazine) (PE) and MGF-Ct24E-modified poly(ethylenediaminetetraacetic dianhydride-co-piperazine) (PEM) showed good antibacterial activity. Considering their different applications, the effects of time, pH, and inoculation concentration of these antibacterials against Escherichia coli (E. coli) in unique environments were evaluated in this study. The results indicated that the MIC and MBC values of the polymers increased after the introduction of MGF-Ct24E into PE, but the two types of polymers still exhibited good antibacterial activity in a short time period under acidic conditions. In addition, we investigated the effect of the piperazine polymers on bacterial cell structure. It was clear that PE and PEM could destroy the bacterial cell wall, cell membrane and DNA, and their specific mechanism may be different. For PE, its carboxyl group could react with peptidoglycans on the E.coli cell wall to form holes on the bacterial surface, allowing PE to penetrate into the bacterial cell to damage DNA. For PEM, the alkaline MGF-Ct24E could adsorb E.coli and make it shrink, meanwhile, the PE component created small holes on the bacterial walls and membranes, and inserted into the bacteria to result in bactericidal effect. These findings reveal the potential usefulness of PE and PEM in biomedical applications. 相似文献
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Many efficient exact branch and bound maximum clique solvers use approximate coloring to compute an upper bound on the clique number for every subproblem. This technique reasonably promises tight bounds on average, but never tighter than the chromatic number of the graph.Li and Quan, 2010, AAAI Conference, p. 128–133 describe a way to compute even tighter bounds by reducing each colored subproblem to maximum satisfiability problem (MaxSAT). Moreover they show empirically that the new bounds obtained may be lower than the chromatic number.Based on this idea this paper shows an efficient way to compute related “infra-chromatic” upper bounds without an explicit MaxSAT encoding. The reported results show some of the best times for a stand-alone computer over a number of instances from standard benchmarks. 相似文献
88.
For the analysis of noise problems in medium-to-high frequency ranges, the energy flow boundary element method (EFBEM) has been studied. EFBEM is numerical analysis method of energy flow analysis (EFA), and solves energy governing equations using a boundary element method in complex structures. Based on EFBEM, a noise prediction software, “noise analysis system by energy flow analysis” (NASEFA), was developed. For effective maintenance, NASEFA is composed of three main modules: the translator, the model converter, and the main solver. The translator changes the FE model to the NASEFA BE model, and the model converter changes the BE model to an EFBE model, including various data, such as structural materials, medium properties, sources, and boundary conditions. NASEFA then solves the acoustic energy density and intensity on boundary and in the field. Moreover, it analyzes interior and exterior noise problems for single and multiple domains in two and three dimensions. Finally, for the validation of the software developed, interior and exterior noise predictions of various structures were performed. The results obtained with NASEFA were compared with those of the commercial SEA program and experiment. From these comparative studies, the usefulness of NASEFA was established. 相似文献
89.
Sustainable management of groundwater-dependent vegetation (GDV) requires the accurate identification of GDVs, characterisation of their water use dynamics and an understanding of associated errors. This paper presents sensitivity and uncertainty analyses of one GDV mapping method which uses temperature differences between time-series of modelled and observed land surface temperature (LST) to detect groundwater use by vegetation in a subtropical woodland. Uncertainty in modelled LST was quantified using the Jacobian method with error variances obtained from literature. Groundwater use was inferred where modelled and observed LST were significantly different using a Student's t-test. Modelled LST was most sensitive to low-range wind speeds (<1.5 m s−1), low-range vegetation height (<=0.5 m), and low-range leaf area index (<=0.5 m2 m−2), limiting the detectability of groundwater use by vegetation under such conditions. The model-data approach was well-suited to detection of GDV because model-data errors were lowest for climatic conditions conducive to groundwater use. 相似文献
90.
A pair of gyradius ratios, defined from the principal radii of gyration, are used to generate a dimension map that describes the geometry of molecular aggregates in water and in organic solvents. Molecular dynamics simulations were performed on the aggregation of representative biomolecules and polyaromatic compounds to demonstrate application of the dimension map. It was shown that molecular aggregate data on the dimension map were bounded by two boundary curves, and that the map could be separated into three regions representing three groups of structures: one-dimensional rod-like structures; two-dimensional planar structures or short-cylinder-like structures; and three-dimensional sphere-like structures. Examining the location of the aggregates on the dimension map and how the location changes with solvent type and solute material parameter provides a simple yet effective way to infer the aggregation manner and to study solubility and mechanism of aggregation. 相似文献